Temperature-Driven Pinned Layer Magnetization Reversal in Exchange Biased Fe₃O₄/Alq₃/Co/CoO Hybrid Spin Valve

In this article, we provide an initial qualitative description of the basic magnetization reversal processes behind temperature and cooling field-dependent exchange bias effect at Co/CoO interface of Fe
₃
O
₄
/Alq
₃
/Co/CoO/Au hybrid spin valve (SV) device structure. The exchange field at Co/CoO interface is observed to be inversely proportional to temperature, indicating enhanced magnetic field sensitivity of Co reverse domain nucleation at the high-temperature region. The exchange field, at constant temperature, is found to be insensitive to change in the cooling field, which may be due to efficient ferromagnetic coupling at the Co/CoO interface of the device. Sudden decrease of exchange field with training cycle number (n) has been observed at lower values of n, which may be attributed to rearrangement of Co pinned layer spin configuration toward equilibrium. Interestingly, incorporation of antiferromagnetic CoO layer has not been observed to bring any change in magnetoresistance (MR) behavior of the exchange biased SV device, which shows a two-step switching pattern of MR at 100 K.